6 Zodiac Signs Most Likely To Be Libra Soulmate AstrologifyLibra love perfect horoscope signs are gemini, water bearer, and aries. When it comes to matters of the heart, Libra seeks harmony and compatibility above all else. The Twins can bring stimulation and fun to the bond, while The Water Bearer shares Libra's appreciation for mind and creativity. The Ram, known for their passion, can ignite a spark in Libra's soul. Libra and these signs create a well-rounded and rewarding union.